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Pengbo Wang, Yibo Wang, Zhaoping Shi, Hongxiang Wu, Jiahao Yang, Jing Ni, Junjie Ge, Changpeng Liu, Wei Xing. Ruthenium-based metal oxide for acidic oxygen evolution reaction: advances and challenges[J]. Energy Lab, 2023, 1(3): 220018. doi: 10.54227/elab.20220018
Citation: Pengbo Wang, Yibo Wang, Zhaoping Shi, Hongxiang Wu, Jiahao Yang, Jing Ni, Junjie Ge, Changpeng Liu, Wei Xing. Ruthenium-based metal oxide for acidic oxygen evolution reaction: advances and challenges[J]. Energy Lab, 2023, 1(3): 220018. doi: 10.54227/elab.20220018
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REVIEW ARTICLE

Ruthenium-based metal oxide for acidic oxygen evolution reaction: advances and challenges

More Information
  • 1.

    Laboratory of Advanced Power Sources, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, China

  • 2.

    School of Applied Chemistry and Engineering, University of Science and Technology of China, Hefei 230026, China

  • 3.

    Jilin Province Key Laboratory of Low Carbon Chemical Power Sources, Changchun 130022, China

  • 4.

    State Key Laboratory of Electroanalytical Chemistry, Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, Changchun 130022, China

  • Corresponding authors: gejunjie@ustc.edu.cn; liuchp@ciac.ac.cn; xingwei@ciac.ac.cn

    • § These authors contributed equally to this work.

    Abstract

  • Utilizing proton exchange membrane water electrolyzers (PEMWE) to produce hydrogen is a promising way to provide clean energy, reduce carbon emissions and improve the utilization rate of renewable energy. The slow kinetics of oxygen evolution reaction (OER) at the anode is considered to be the crucial obstacle to its conversion efficiency. Due to the strong acidic and oxidizing environment of OER reaction, it is essential to develop electrocatalyst with high activity and high stability to reduce the high kinetic barrier of OER and improve the reaction rate. Among them, Ru-based catalysts have outstanding catalytic activity and relatively low price, which has aroused great interest in its practical application. Many Ru-based catalysts with superior performance have been developed in recent years. In this review, we mainly focus on the development of Ru-based catalysts towards OER, with OER mechanisms discussed first, followed by discussion in the factors affecting the catalytic performance, and then introduce current research progress of Ru-based catalysts under acidic conditions. We finally conclude the prospect of the development direction of Ru-based catalysts in the future, hopefully guiding further development of Ru-based catalysts towards real world operation.


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    • Author Biographies
  • Pengbo Wang received his BS from Nanjing University of Science and Technology, China, in 2021. Currently, he is a master student at Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, China. under the supervision of Professor Changpeng Liu. Now his research focuses on water electrolysis technology and its microscopic reaction mechanism.
    Yibo Wang received his BS from Zhengzhou University, China, in 2018. Currently, he is an MA candidate in Physical Chemistry under the supervision of Prof. Wei Xing at the Changchun Institute of Applied Chemistry, Chinese Academy of Sciences, China. Now his research focuses on water electrolysis technology and its microscopic reaction mechanism.
    Junjie Ge received her Ph.D. in physical chemistry from the Chinese Academy of Sciences in 2010. She worked at the University of South Carolina and Hawaii Natural Energy Institute as a postdoc and joined Changchun Institute of Applied Chemistry in March 2015 as a full professor. Her research interests include fuel cells, nanoscience, catalysis, and electrochemistry. She has published over 30 peer-reviewed papers and several posters, abstracts and presentations. She is also acting as a referee for several top journals in the field related to catalysis, electro-chemistry, and fuel cells.
    Changpeng Liu received his Ph.D. in Physical Chemistry in 2002 and was appointed as a professor at the Changchun Institute of Applied Chemistry in 2012. He has been in charge of and taken part in several relevant fuel cell projects (e.g. 863 programs and 973 programs China). Liu’s research focuses on the technology and performance of catalysts, electrode MEA and stacks.
    Wei Xing is currently director of the Laboratory of Advanced Power Sources in Changchun Institute of Applied Chemistry (CIAC). After receiving his Ph.D. in Physical Chemistry, at CIAC in 1995, he worked at the Hong Kong Productivity Council (HKPC), researching the electrochemical treatment of metal surfaces. In 2001, he joined CIAC as a professor and devoted his work to development of advanced chemical power sources. He has published over 150 papers in peer-reviewed journals and has applied for over 30 patents. His research areas currently involve proton exchange membrane fuel cells from fundamental electro-catalytic processes to relevant fuel cell assembly and testing.
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Received Date:  22 December 2022
Revised Date:  16 March 2023
Accepted Date:  24 April 2023
Available Online:  19 May 2023
Publish Date:  28 July 2023

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