Yi Yang, Lei Xu, Chong Yan, Jiaqi Huang, Qiang Zhang. Towards the intercalation and lithium plating mechanism for high safety and fast-charging lithium-ion batteries: a review[J]. Energy Lab, 2023, 1(1): 220011. doi: 10.54227/elab.20220011
Citation: Yi Yang, Lei Xu, Chong Yan, Jiaqi Huang, Qiang Zhang. Towards the intercalation and lithium plating mechanism for high safety and fast-charging lithium-ion batteries: a review[J]. Energy Lab, 2023, 1(1): 220011. doi: 10.54227/elab.20220011

REVIEW ARTICLE

Towards the intercalation and lithium plating mechanism for high safety and fast-charging lithium-ion batteries: a review

More Information
  • Corresponding authors: yanc@bit.edu.cn; zhang-qiang@mails.tsinghua.edu.cn
  • The ever-increasing demand of portable electronics and electric vehicles has consistently promoted the development of lithium-ion batteries (LIBs) in the direction of higher energy density, higher safety, and faster charging. However, present high-energy LIBs are insufficient to sustain extra-fast power input without adverse consequences, which is mainly affected by the lithium (Li) plating on graphite electrode. The goal of this review is to enable graphite anode to support higher current and improve safety by ameliorating undesired Li plating from fundamentals and detections. Hence, the interaction, containing solid electrolyte interphase formation, Li+ intercalation/plating behavior, between graphite and Li+ be discussed in depth. Besides, the cognitive process of Li+ intercalation/plating kinetics as well as the inner mechanisms of Li plating especially in 3 extreme conditions (high state-of-charge, high charging-rate, and low temperature) are highly desirable to investigate Li plating comprehensively. Meanwhile, issues induced by Li plating, detection methods of Li deposition and knowledge gaps are identified for the follow-up research directions of Li plating in LIBs.


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  • Yi Yang received his B.E. degree from Sun Yue-Qi Honors College in China University of Mining and Technology (2020). Presently, he is a Ph.D. student in Advanced Research Institute of Multidisciplinary Science (ARIMS), Beijing Institute of Technology, under the supervision of Prof. Jia-Qi Huang. His current research interests focus on the fast charging and the Li plating issue of graphite anode.
    Lei Xu received his B.E. degree in Chemical Engineering from Beijing Institute of Technology in 2018. Then, he joined Prof. Jia-Qi Huang’s group as a Ph.D. student at Advanced Research Institute of Multidisciplinary Science (ARIMS), Beijing Institute of Technology. His research interest focuses on the interfacial behavior towards fast-charging batteries and the safety of lithium-ion batteries.
    Chong Yan received his bachelor’s (2013) and master’s (2017) degrees from Henan Normal University and got his PhD degrees (2020) at Beijing Institute of Technology. He had done his postdoctoral research at Tsinghua University for two years. He is currently an associate professor in Advanced Research Institute of Multi-disciplinary Science (ARIMS) in Beijing Institute of Technology. His research focuses on the fast-charging technology of lithium-ion batteries and the Nano-sized formation mechanism of electrode/electrolyte interface.
    Jia-Qi Huang received his BEng (2007) and PhD (2012) degrees in Chemical Engineering from Tsinghua University, China. He is currently a professor in Advanced Research Institute of Multi-disciplinary Science (ARIMS) in Beijing Institute of Technology. His research interests focus on the interface phenomenon and design strategies for high-energy density rechargeable batteries, including Li–S batteries, Li metal batteries, etc.
    Qiang Zhang received his bachelor’s and PhD degrees from Tsinghua University in 2004 and 2009, respectively. After spending some time at Case Western Reserve University, USA, and Fritz Haber Institute of the Max Planck Society, Germany, he was appointed as a faculty member at Tsinghua University in 2011. His interests are focused on energy materials, including Li–S batteries, Li metal anode, 3D graphene, and electro-catalysts. He was awarded The National Science Fund for Distinguished Young Scholars, Young Top-Notch Talent from China, and Newton Advanced Fellowship from the Royal Society, UK. Currently, he is an associate editor of the Journal of Energy Chemistry and Energy Storage Materials.
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