Hassina Tabassum, Shreya Mukherjee, Thomas O'Carroll, Tianjie Qiu, Xiaoxuan Yang, Ruqiang Zou, Gang Wu. High-entropy nanomaterials for electrochemical energy conversion and storage[J]. Energy Lab, 2023, 1(1): 220006. doi: 10.54227/elab.20220006
Citation: Hassina Tabassum, Shreya Mukherjee, Thomas O'Carroll, Tianjie Qiu, Xiaoxuan Yang, Ruqiang Zou, Gang Wu. High-entropy nanomaterials for electrochemical energy conversion and storage[J]. Energy Lab, 2023, 1(1): 220006. doi: 10.54227/elab.20220006

REVIEW ARTICLE

High-entropy nanomaterials for electrochemical energy conversion and storage

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  • Corresponding authors: hassinat@buffalo.edu; rzou@pku.edu.cn; gangwu@buffalo.edu
  • High entropy materials (HEMs) with a single-phase structure have introduced a brand-new area of research in electrochemical energy conversion and storage devices. The fusion of divergent elements has been found to produce synergistic effects with advanced physicochemical phenomena. As such, heterometallic equiatomic proportion-based nanomaterials with stabilized configurational mixed entropy exhibit distinguished characteristics to enhance electrode catalytic activity and storage capability. This critical review summarizes the recent advances in developing HEMs at the nanoscale using different synthetic technologies. The most popular types of HEMs are high entropy alloys (HEAs) and high entropy oxides (HEOs), both of which present tunable structural properties. This review pays particular attention to recapitulating the necessary considerations to obtain HEAs effective for water splitting, fuel cell operation, CO2 reduction reactions, and energy storage applications. The demonstrated examples bestow a deep understanding of efficient HEM utilization as electrocatalysts and electrodes for charge storage devices. Finally, challenges and future perspectives pertaining to HEMs adoption as desirable materials for electrochemical energy conversion and storage devices will be discussed.


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  • Hassina Tabassum is a Postdoctoral Associate at the University at Buffalo, the State University of New York (SUNY), USA. Before this, she was a Boya Postdoctoral fellow at Peking university. She has published several high-quality research articles. Her publications have been cited more than 3400 times with H-index of 29. She is several award recipients, including Peking University’s best academic award 2016, Top Ten Best Young Researchers Award of Peking University 2017, Joule Star Talk Award 2019, and the International young scientist funding award 2020. Her research interests are based on the fabrication of advanced nanomaterials for electrochemical energy conversion and storage devices.
    Xiaoxuan Yang was a visiting Ph.D. student at the University at Buffalo, the State University of New York (SUNY). She obtained her Ph.D. at Northeast Normal University in 2021. Currently, she is a postdoc at Zhejiang University. Her research interests mainly focus on the design, synthesis, and characterization of functional nanomaterials for electrochemical energy storage and conversion.
    Ruqiang Zou is currently a full professor and dean of School of Materials Science and Engineering, Peking University, P. R. China. He received his Ph.D. in engineering in 2008 from Kobe University and the National Institute of Advanced Industrial Science and Technology, Japan. He held the JSPS younger scientist during his doctoral course and was a director's postdoc fellow at Los Alamos National Laboratory from 2008 to 2010. He was awarded the Outstanding Young Scientist Foundation of NSFC and Changjiang Scholar. His research interests focus on the controllable preparation of hierarchically porous functional materials for energy and environmental applications.
    Gang Wu is a Professor of Chemical Engineering at the University at Buffalo (UB), SUNY. He obtained his B.S. in 1997 and Ph.D. in 2004 at the Harbin Institute of Technology. After postdoctoral training at Tsinghua University, the University of South Carolina, and Los Alamos National Laboratory (LANL), he became a staff scientist at LANL in 2010. He joined UB in 2014 as an assistant professor and was promoted to tenured associate professor in 2018 and a full professor in 2020. He has published more than 300 papers with 39000 citations, leading an H-index of 106. He is a Highly Cited Researcher ranked by Thomson Reuters, Clarivate Analytics since 2018. His research interests are electrochemical energy science and technology, with an emphasis on advanced electrocatalysis for fuel cells, water electrolzyers, CO2 reduction, and chemical electrosynthesis.
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